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Zoloft (Sertraline HCl) is one of a class of Thyroid medication levothyroxine antidepressant drugs known as selective serotonin reuptake inhibitors (SSRIs). These drugs work by increasing the amount of serotonin that is available in the brain. Serotonin is involved in regulating mood and Thyroid medication levothyroxine general feelings of well-being.